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EFFICIENT CONTAMINANT REMOVAL FROM LIQUID DIGESTATE OF PIG MANURE BY CHEMICAL PRECIPITATION AND CO MINERALIZATION

《农业科学与工程前沿（英文）》 2023年 第10卷 第3期   页码 479-491 doi: 10.15302/J-FASE-2023480

摘要：

● LFD was treated by fly ash-based chemical precipitation and CO2 mineralization.

关键词： anaerobic digestion     chemical oxygen demand     fly ash     ion removal     total phosphate    

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Effect of short-term atrazine addition on the performance of an anaerobic/anoxic/oxic process

Changyong WU, Xiaoling LI, Zhiqiang CHEN, Yongzhen PENG,

《环境科学与工程前沿（英文）》 2010年 第4卷 第2期   页码 150-156 doi: 10.1007/s11783-010-0020-9

摘要： In this study, an anaerobic/anoxic/oxic (AO) wastewater treatment process was implemented to treat domestic wastewater with short-term atrazine addition. The results provided an evaluation on the effects of an accidental pollution on the operation of a wastewater treatment plant (WWTP) in relation to Chemical Oxygen Demand (COD) and biological nutrient removal. Domestic wastewater with atrazine addition in 3 continuous days was treated when steady biological nutrient removal was achieved in the AO process. The concentrations of atrazine were 15, 10, and 5mg·L on days 1, 2 and 3, respectively. The results showed that atrazine addition did not affect the removal of COD. The specific NH NO reduction rate decreased slightly due to the short-term atrazine addition. However, it did not affect the nitrogen removal due to the high nitrification and denitrification capacity of the system. Total nitrogen (TN) removal was steady, and more than 70% was removed during the period studied. The phosphorus removal rate was not affected by the short-term addition of atrazine under the applied experimental conditions. However, more poly-hydroxy-alkanoate (PHA) was generated and utilized during atrazine addition. The results of the oxygen uptake rate (OUR) showed that the respiration of nitrifiers decreased significantly, while the activity of carbon utilizers had no obvious change with the atrazine addition. Atrazine was not removed with the AO process, even via absorption by the activated sludge in the process of the short-term addition of atrazine.

关键词： biological nutrient removal     atrazine     anaerobic/anoxic/oxic (A2O) process     oxygen demand removal     oxygen uptake rate (OUR)    

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polyhydroxyalkanoates and glycogen transformations: Key aspects to biologic nitrogen and phosphorus removalin low dissolved oxygen systems

Hongjing LI, Yinguang CHEN

《环境科学与工程前沿（英文）》 2011年 第5卷 第2期   页码 283-290 doi: 10.1007/s11783-010-0243-9

摘要： In this paper, a study was conducted on the effect of polyhydroxyalkanoates (PHA) and glycogen transformations on biologic nitrogen and phosphorus removal in low dissolved oxygen (DO) systems. Two laboratory-scale sequencing batch reactors (SBR1 and SBR2) were operating with anaerobic/aerobic (low DO, 0.15–0.45 mg·L ) configurations, which cultured a propionic to acetic acid ratio (molar carbon ratio) of 1.0 and 2.0, respectively. Fewer poly-3-hydroxybutyrate (PHB), total PHA, and glycogen transformations were observed with the increase of propionic/acetic acid, along with more poly-3-hydroxyvalerate (PHV) and poly-3-hydroxy-2-methyvalerate (PH2MV) shifts. The total nitrogen (TN) removal efficiency was 68% and 82% in SBR1 and SBR2, respectively. In the two SBRs, the soluble ortho-phosphate (SOP) removal efficiency was 94% and 99%, and the average sludge polyphosphate (poly-P) content (g·g-MLVSS ) was 8.3% and 10.2%, respectively. Thus, the propionic to acetic acid ratio of the influent greatly influenced the PHA form and quantity, glycogen transformation, and poly-P contained in activated sludge and further determined TN and SOP removal efficiency. Moreover, significant correlations between the SOP removal rate and the (PHV+ PH2MV)/PHA ratio were observed ( >0.99). Accordingly, PHA and glycogen transformations should be taken into account as key components for optimizing anaerobic/aerobic (low DO) biologic nitrogen and phosphorus removal systems.

关键词： low dissolved oxygen (DO)     biological nitrogen and phosphorus removal     polyhydroxyalkanoates (PHA)     glycogen    

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Mercury removal from flue gas using nitrate as an electron acceptor in a membrane biofilm reactor

《环境科学与工程前沿（英文）》 2022年 第16卷 第2期 doi: 10.1007/s11783-021-1454-y

摘要：

Membrane bioreactor achieved mercury removal using nitrate as an electron acceptor.

关键词： Mercury removal     Oxygen     Ferrous sulfide     Transformation of mercury     Microbial community    

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The treatment of black-odorous water using tower bipolar electro-flocculation including the removal ofphosphorus, turbidity, sulfion, and oxygen enrichment

Huan He, Qinjin Yu, Chaochao Lai, Chen Zhang, Muhan Liu, Bin Huang, Hongping Pu, Xuejun Pan

《环境科学与工程前沿（英文）》 2021年 第15卷 第2期 doi: 10.1007/s11783-020-1310-5

摘要： Abstract • An innovative bubble column tower BPE was designed to treat the black-odorous water. • PO43−, S2− and turbidity were removed, and dissolved oxygen was enriched in the BPE. • An aluminum bipolar electrode gave the best oxygen enrichment and pollutant removal. • Changes of microorganisms confirmed the improvement in water quality achieved. The large amount of municipal wastewater discharged into urban rivers sometimes exceeds the rivers’ self-purification capacity leading to black-odorous polluted water. Electro-flocculation has emerged as a powerful remediation technology. Electro-flocculation in a bubble column tower with a bipolar electrode (BPE) was tested in an attempt to overcome the high resistance and weak gas-floatation observed with a monopolar electrode (MPE) in treating such water. The BPE reactor tested had a Ti/Ta2O5-IrO2 anode and a graphite cathode with an iron or aluminum bipolar electrode suspended between them. It was tested for its ability to reduce turbidity, phosphate and sulphion and to increase the concentration of dissolved oxygen. The inclusion of the bipolar electrode was found to distinctly improved the system’s conductivity. The system’s electro-flocculation and electrical floatation removed turbidity, phosphate and sulphion completely, and the dissolved oxygen level improved from 0.29 to 6.28 mg/L. An aluminum bipolar electrode performed better than an iron one. Changes in the structure of the microbial community confirmed a significant improvement in water quality.

关键词： Black-odorous water     Bipolar electrodes     Flocculation     Floatation     Oxygen enrichment     Turbidity    

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Control of sludge settleability and nitrogen removal under low dissolved oxygen condition

Zhaoxu PENG, Yongzhen PENG, Zhenbo YU, Xuliang LIU, Xiaoling LI, Randeng WANG

《环境科学与工程前沿（英文）》 2012年 第6卷 第6期   页码 884-891 doi: 10.1007/s11783-012-0408-9

摘要： Low dissolved oxygen (DO) is an energy-saving condition in activated sludge process. To investigate the possible application of limited filamentous bulking (LFB) in sequencing batch reactor (SBR), two lab-scale SBRs were used to treat synthetic domestic wastewater and real municipal wastewater, respectively. The results showed that prolonging low DO aeration duration and setting pre-anoxic (anaerobic) phase were effective strategies to induce and inhibit filamentous sludge bulking, respectively. According to the sludge settleability, LFB could be maintained steadily by adjusting operation patterns. Filamentous bacteria content and sludge volume index (SVI) were likely correlated. SVI fluctuated dramatically within a few cycles when around 200 mL·g , where altering operation pattern could change sludge settleability in spite of the unstable status of activated sludge system. Energy consumption by aeration reduced under low DO LFB condition, whereas the nitrification performance deteriorated. However, short-cut nitrification and simultaneous nitrification denitrification (SND) were prone to take place under such conditions. When the cycle time kept constant, the anoxic (anaerobic) to aerobic time ratio was determining factor to the SND efficiency. Similarity keeping aerobic time as constant, the variation trends of SND efficiency and specific SND rate were uniform. SBR is a promising reactor to apply the LFB process in practice.

关键词： limited filamentous bulking     sequencing batch reactor     sludge settleability     sludge volume index     simultaneous nitrification denitrification    

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Removal of dissolved oxygen from water using a Pd-resin based catalytic reactor

Wenxin SHI, Chongwei CUI, Liye ZHAO, Shuili YU, Xia YUN

《化学科学与工程前沿（英文）》 2009年 第3卷 第1期   页码 107-111 doi: 10.1007/s11705-009-0154-0

摘要： The removal of dissolved oxygen (DO) from water was studied experimentally in a Pd-resin base catalyst reactor using purified hydrogen gas as a reducing agent. The effects of various operating conditions, such as hydrogen and water flow rates, height of the catalytic resin bed, temperature, pH value and run time, on the removal of DO, had been studied extensively. The results shows that DO could be removed by the reactor from ppm to ppb levels at ambient temperature. Increases of temperature, H gas rate and the height of the catalytic resin were helpful to improve the DO removal rate. The change of pH value from 4 to 12 resulted in no effect on DO removal. Reaction time was the key factor to control the DO removal efficiency. Only when the reaction time was longer than 2.3 minutes under the experimental conditions, could a very low DO level be achieved.

关键词： dissolved oxygen     palladium     catalytic reactor     hydrogen     resin    

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Flocculation behaviors of a novel papermaking sludge-based flocculant in practical printing and dyeing wastewater treatment

《环境科学与工程前沿（英文）》 2021年 第15卷 第5期 doi: 10.1007/s11783-021-1390-x

摘要：

•PSBF performed better than PAC and PAM in CODCr removals.

关键词： Practical wastewater treatment     Commercial coagulant/flocculant     Secondary coagulation-flocculation process     Chemical oxygen demand     Coagulation-flocculation mechanism    

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Water quality prediction of copper-molybdenum mining-beneficiation wastewater based on the PSO-SVR model

《环境科学与工程前沿（英文）》 2023年 第17卷 第8期 doi: 10.1007/s11783-023-1698-9

摘要：

● Data acquisition and pre-processing for wastewater treatment were summarized.

关键词： Chemical oxygen demand     Mining-beneficiation wastewater treatment     Particle swarm optimization     Support vector regression     Artificial neural network    

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MILP synthesis of separation processes for waste oil-in-water emulsions treatment

Zorka N. Pintarič,Gorazd P. Škof,Zdravko Kravanja

《化学科学与工程前沿（英文）》 2016年 第10卷 第1期   页码 120-130 doi: 10.1007/s11705-016-1559-1

摘要： This paper presents a novel synthesis method for designing integrated processes for oil-in-water (O/W) emulsions treatment. General superstructure involving alternative separation technologies is developed and modelled as a mixed integer linear programming (MILP) model for maximum annual profit. Separation processes in the superstructure are divided into three main sections of which the pretreatment and final treatment are limited to the selection of one alternative (or bypass) only, while within the intermediate section various combinations of different technologies in series can be selected. Integrated processes composed of selected separation techniques for given ranges of input chemical oxygen demand (COD) can be proposed by applying parametric analyses within the superstructure approach. This approach has been applied to an existing industrial case study for deriving optimal combinations of technologies for treating diverse oil-in-water emulsions within the range of input COD values between 1000 mg?L and 145000 mg?L . The optimal solution represents a flexible and profitable process for reducing the COD values below maximal allowable limits for discharging effluent into surface water.

关键词： oil-in-water emulsion     chemical oxygen demand     superstructure     process synthesis     MILP    

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Effects of cultivation strategies on the cultivation of Chlorella sp. HQ in photoreactors

Xiaoya Liu, Yu Hong, Peirui Liu, Jingjing Zhan, Ran Yan

《环境科学与工程前沿（英文）》 2019年 第13卷 第5期 doi: 10.1007/s11783-019-1162-z

摘要： Heterotrophic cultivation caused high level of ROS and high lipids accumulation. HMTC is the best culture strategy for improving the microalgal biomass. Chlorella sp. HQ had great nutrient removal capacity under five culture strategies. The effects of cultivation strategies (including autotrophic cultivation (AC), heterotrophic cultivation (HC), fed-batch cultivation (FC), heterotrophic+ autotrophic two-stage cultivation (HATC), and heterotrophic+ mixotrophic two-stage cultivation (HMTC)) on the growth and lipid accumulation of Chlorella sp. HQ and its total nitrogen (TN) and total phosphorus (TP) removal in secondary effluent were investigated in column photoreactors. The results showed that the TN and TP removal rates ranged between 93.72%–95.82% and 92.73%–100%, respectively, under the five different strategies. The microalgal growth potential evaluated by the maximal growth rate (Rmax) was in the order of HMTC>HC>FC>AC>HATC. The values of biomass, total lipid yield, triacylglycerols (TAGs) yield, and total lipid content of the microalga cultivated in the last 5 d increased significantly, but the TAGs productivities of the five strategies were lower than those in the first 7 d. Compared with all the other cultivation strategies, the TAGs productivity and yield after 12 d of cultivation under the heterotrophic condition reached the highest values accompanying the highest level of intracellular reactive oxygen species (ROS), in which the TAGs yield reached 40.81 mg/L at the end of the cultivation period. The peaks in TAGs yield and ROS level suggested that HC was beneficial for lipids accumulation via regulating the cellular redox status and exerting ROS stress on microalgal cells. In summary, HMTC was the best cultivation strategy for improving the microalgal biomass and HC was the best strategy for microalgal TAGs accumulation to produce biodiesel.

关键词： Chlorella sp. HQ     Cultivation strategy     lipids     Nitrogen removal     Phosphorus removal     Reactive oxygen species    

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Heterometallic cluster-based organic frameworks as highly active electrocatalysts for oxygen reductionand oxygen evolution reaction: a density functional theory study

《化学科学与工程前沿（英文）》 2023年 第17卷 第5期   页码 570-580 doi: 10.1007/s11705-022-2247-y

摘要： Recently, metal–organic frameworks are one of the potential catalytic materials for electrocatalytic applications. The oxygen reduction reaction and oxygen evolution reaction catalytic activities of heterometallic cluster-based organic frameworks are investigated using density functional theory. Firstly, the catalytic activities of heterometallic clusters are investigated. Among all heterometallic clusters, Fe2Mn–Mn has a minimum overpotential of 0.35 V for oxygen reduction reaction, and Fe2Co–Co possesses the smallest overpotential of 0.32 V for oxygen evolution reaction, respectively 100 and 50 mV lower than those of Pt(111) and RuO2(110) catalysts. The analysis of the potential gap of Fe2M clusters indicates that Fe2Mn, Fe2Co, and Fe2Ni clusters possess good bifunctional catalytic activity. Additionally, the catalytic activity of Fe2Mn and Fe2Co connected through 3,3′,5,5′-azobenzenetetracarboxylate linker to form Fe2M–PCN–Fe2M is explored. Compared with Fe2Mn–PCN–Fe2Mn, Fe2Co–PCN–Fe2Co, and isolated Fe2M clusters, the mixed-metal Fe2Co–PCN–Fe2Mn possesses excellent bifunctional catalytic activity, and the values of potential gap on the Mn and Co sites of Fe2Co–PCN–Fe2Mn are 0.69 and 0.70 V, respectively. Furthermore, the analysis of the electron structure indicates that constructing a mixed-metal cluster can efficiently enhance the electronic properties of the catalyst. In conclusion, the mixed-metal cluster strategy provides a new approach to further design and synthesize high-efficiency bifunctional electrocatalysts.

关键词： bimetallic metal–organic frameworks     bifunctional electrocatalyst     density functional theory     oxygen reduction reaction     oxygen evolution reaction    

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Understanding the demand predictability of bike share systems: A station-level analysis

《工程管理前沿（英文）》   页码 551-565 doi: 10.1007/s42524-023-0279-8

摘要： Predicting demand for bike share systems (BSSs) is critical for both the management of an existing BSS and the planning for a new BSS. While researchers have mainly focused on improving prediction accuracy and analysing demand-influencing factors, there are few studies examining the inherent randomness of stations’ observed demands and to what degree the demands at individual stations are predictable. Using Divvy bike-share one-year data from Chicago, USA, we measured demand entropy and quantified the station-level predictability. Additionally, to verify that these predictability measures could represent the performance of prediction models, we implemented two commonly used demand prediction models to compare the empirical prediction accuracy with the calculated entropy and predictability. Furthermore, we explored how city- and system-specific temporally-constant features would impact entropy and predictability to inform estimating these measures when historical demand data are unavailable. Our results show that entropy of demands across stations is polarized as some stations exhibit high uncertainty (a low entropy of 0.65) and others have almost no check-out demand uncertainty (a high entropy of around 1.0). We also validated that the entropy and predictability are a priori model-free indicators for prediction error, given a sequence of bike usage demands. Lastly, we identified that key factors contributing to station-level entropy and predictability include per capita income, spatial eccentricity, and the number of parking lots near the station. Findings from this study provide more fundamental understanding of BSS demand prediction, which can help decision makers and system operators anticipate diverse station-level prediction errors from their prediction models both for existing stations and for new ones.

关键词： bike share systems     demand prediction     prediction errors     machine learning     entropy    

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Optimal locations of monitoring stations in water distribution systems under multiple demand patterns: a flaw of demand coverage method and modification

Shuming LIU, Wenjun LIU, Jinduan CHEN, Qi WANG

《环境科学与工程前沿（英文）》 2012年 第6卷 第2期   页码 204-212 doi: 10.1007/s11783-011-0364-9

摘要： A flaw of demand coverage method in solving optimal monitoring stations problem under multiple demand patterns was identified in this paper. In the demand coverage method, the demand coverage of each set of monitoring stations is calculated by accumulating their demand coverage under each demand pattern, and the impact of temporal distribution between different time periods or demand patterns is ignored. This could lead to miscalculation of the optimal locations of the monitoring stations. To overcome this flaw, this paper presents a Demand Coverage Index (DCI) based method. The optimization considers extended period unsteady hydraulics due to the change of nodal demands with time. The method is cast in a genetic algorithm framework for integration with Environmental Protection Agency Net (EPANET) and is demonstrated through example applications. Results show that the set of optimal locations of monitoring stations obtained using the DCI method can represent the water quality of water distribution systems under multiple demand patterns better than the one obtained using previous methods.

关键词： demand coverage     monitoring     optimization     water distribution network     water quality    

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Electricity demand, GDP and employment: evidence from Italy

Cosimo MAGAZZINO

《能源前沿（英文）》 2014年 第8卷 第1期   页码 31-40 doi: 10.1007/s11708-014-0296-8

摘要： This paper applies time series methodologies to examine the causal relationship among electricity demand, real per capita GDP and total labor force for Italy from 1970 to 2009. After a brief introduction, a survey of the economic literature on this issue is reported, before discussing the data and introducing the econometric techniques used. The results of estimation indicate that one cointegrating relationship exists among these variables. This equilibrium relation implies that, in the long-run, GDP and labor force are correlated negatively, as well as GDP and electricity. Moreover, there is a bi-directional Granger causality flow between real per capita GDP and electricity demand; while labor force does not Granger-cause neither real per capita GDP nor electricity demand. This implies that electricity demand and economic growth are jointly determined at the same time for the Italian case. The forecast error variance decomposition shows that forecast errors in real per capita GDP are mainly caused by the uncertainty in GDP itself, while forecast errors in labor force are mainly resulted from the labor force itself, although aggregate income and electricity are important, too.

关键词： energy policies     electricity demand     GDP     labor force     stationarity     structural breaks     cointegration     causality     Italy    

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标题 作者 时间 类型 操作

EFFICIENT CONTAMINANT REMOVAL FROM LIQUID DIGESTATE OF PIG MANURE BY CHEMICAL PRECIPITATION AND CO MINERALIZATION

期刊论文

Effect of short-term atrazine addition on the performance of an anaerobic/anoxic/oxic process

Changyong WU, Xiaoling LI, Zhiqiang CHEN, Yongzhen PENG,

期刊论文

polyhydroxyalkanoates and glycogen transformations: Key aspects to biologic nitrogen and phosphorus removalin low dissolved oxygen systems

Hongjing LI, Yinguang CHEN

期刊论文

Mercury removal from flue gas using nitrate as an electron acceptor in a membrane biofilm reactor

期刊论文

The treatment of black-odorous water using tower bipolar electro-flocculation including the removal ofphosphorus, turbidity, sulfion, and oxygen enrichment

Huan He, Qinjin Yu, Chaochao Lai, Chen Zhang, Muhan Liu, Bin Huang, Hongping Pu, Xuejun Pan

期刊论文

Control of sludge settleability and nitrogen removal under low dissolved oxygen condition

Zhaoxu PENG, Yongzhen PENG, Zhenbo YU, Xuliang LIU, Xiaoling LI, Randeng WANG

期刊论文

Removal of dissolved oxygen from water using a Pd-resin based catalytic reactor

Wenxin SHI, Chongwei CUI, Liye ZHAO, Shuili YU, Xia YUN

期刊论文

Flocculation behaviors of a novel papermaking sludge-based flocculant in practical printing and dyeing wastewater treatment

期刊论文

Water quality prediction of copper-molybdenum mining-beneficiation wastewater based on the PSO-SVR model

期刊论文

MILP synthesis of separation processes for waste oil-in-water emulsions treatment

Zorka N. Pintarič,Gorazd P. Škof,Zdravko Kravanja

期刊论文

Effects of cultivation strategies on the cultivation of Chlorella sp. HQ in photoreactors

Xiaoya Liu, Yu Hong, Peirui Liu, Jingjing Zhan, Ran Yan

期刊论文

Heterometallic cluster-based organic frameworks as highly active electrocatalysts for oxygen reductionand oxygen evolution reaction: a density functional theory study

期刊论文

Understanding the demand predictability of bike share systems: A station-level analysis

期刊论文

Optimal locations of monitoring stations in water distribution systems under multiple demand patterns: a flaw of demand coverage method and modification

Shuming LIU, Wenjun LIU, Jinduan CHEN, Qi WANG

期刊论文

Electricity demand, GDP and employment: evidence from Italy

Cosimo MAGAZZINO

期刊论文